CVEN 6414 Aquatic Surfaces and Particles

Problem Set 4: Adsorption Competition

 

Using Visual MINTEQ, complete the following assignment.

  1. Calculate the competitive adsorption of copper and lead on hydrous ferric oxide (HFO) as a function of pH from pH 2 to 12 using the two-pKa double-layer model.  For HFO, the concentration is 90 mg L-1, the surface area is 600 m2 g-1, the site density is 3 sites nm-2, and the pKaint values are 7.29 and 8.93.  The ionic strength is controlled using 0.1 M NaNO3.  The copper and lead surface complexation constants are listed in Table 6 of Koretsky et al. (2000).

    (a) For total copper and lead concentrations of 10-6 M.
    (b) For total copper of 10-6 M and total lead of 10-7 M.
    (c) For total copper of 10-6 M and total lead of 10-8 M.

    Describe the effect of the competition on copper and lead adsorption as illustrated by the three cases. 
     
  2. Calculate the competitive adsorption of phosphate and arsenate on hydrous ferric oxide (HFO) as a function of pH from pH 2 to 12 using the two-pKa double-layer model.  For HFO, the concentration is 90 mg L-1, the surface area is 600 m2 g-1, the site density is 3 sites nm-2, and the pKaint values are 7.29 and 8.93.  The ionic strength is controlled using 0.1 M NaNO3.  The phosphate and arsenate surface complexation constants are listed in Table 6 of Koretsky et al. (2000).  Notice that multiple surface species exist for both phosphate and arsenate.

    (a) For total phosphate and arsenate concentrations of 10-5 M.
    (b) For total phosphate of 10-5 M and total arsenate of 10-6 M.
    (c) For total phosphate of 10-5 M and total arsenate of 10-7 M.

    Describe the effect of the competition on phosphate and arsenate adsorption as illustrated by the three cases. 

     

Last updated on May 20, 2007 by Joe Ryan